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  • Title: In-situ encapsulation of quantum dots into polymer microspheres.
    Author: Sheng W, Kim S, Lee J, Kim SW, Jensen K, Bawendi MG.
    Journal: Langmuir; 2006 Apr 11; 22(8):3782-90. PubMed ID: 16584256.
    Abstract:
    We have incorporated fluorescent quantum dots (QDs) into polystyrene microspheres using functionalized oligomeric phosphine (OP) ligands. We find that a uniform distribution of quantum dots is loaded inside each polymer bead. Some local close-packing of quantum dots in the beads is attributed to the self-polymerization of the functionalized ligands. The presence of quantum dots disturbs the nucleation and growth processes during the formation of polymer microspheres and results in a wider size distribution of the quantum dot-embedded polystyrene beads than for the control without dots. The change in quantum efficiency of the quantum dots before (approximately 20%) and after (12%) loading into the beads substantiates the protection of oligomeric phosphine ligands yet indicates that the properties of these quantum dots are still affected during processing.
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