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  • Title: Ruthenium hydride-catalyzed addition of aldehydes to dienes leading to beta,gamma-unsaturated ketones.
    Author: Omura S, Fukuyama T, Horiguchi J, Murakami Y, Ryu I.
    Journal: J Am Chem Soc; 2008 Oct 29; 130(43):14094-5. PubMed ID: 18841894.
    Abstract:
    An efficient cross-addition reaction of dienes with aldehydes was developed by using RuHCl(CO)(PPh3)3 as a catalyst to give a wide variety of beta,gamma-unsaturated ketones, where a pi-allylruthenium species, derived from hydroruthenation of diene, may be involved as a key intermediate.
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