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  • Title: Facile fabrication of an efficient oxynitride TaON photoanode for overall water splitting into H2 and O2 under visible light irradiation.
    Author: Abe R, Higashi M, Domen K.
    Journal: J Am Chem Soc; 2010 Sep 01; 132(34):11828-9. PubMed ID: 20443625.
    Abstract:
    The porous oxynitride TaON film electrode prepared on conducting glass (FTO) showed significantly high quantum efficiency (IPCE = ca. 76% at 400 nm at 0.6 V vs Ag/AgCl) in an aqueous Na(2)SO(4) solution, after loading of IrO(2) x nH(2)O nanoparticles as a cocatalyst for water oxidation. Overall water splitting into H(2) and O(2) under visible light was demonstrated using an IrO(2) x nH(2)O-loaded TaON photoanode combined with a Pt electrode under an externally applied bias (0.6-1 V).
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