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  • Title: Application of bifunctional magnetic adsorbent to adsorb metal cations and anionic dyes in aqueous solution.
    Author: Lin YF, Chen HW, Chien PS, Chiou CS, Liu CC.
    Journal: J Hazard Mater; 2011 Jan 30; 185(2-3):1124-30. PubMed ID: 21084161.
    Abstract:
    A magnetic adsorbent, amine-functionalized silica magnetite (NH(2)/SiO(2)/Fe(3)O(4)), has been synthesized to behave as an anionic or cationic adsorbent by adjusting the pH value of the aqueous solution to make amino groups protonic or neutral. NH(2)/SiO(2)/Fe(3)O(4) were used to adsorb copper ions (metal cation) and Reactive Black 5 (RB5, anionic dye) in an aqueous solution in a batch system, and the maximum adsorption were found to occur at pH 5.5 and 3.0, respectively. The adsorption equilibrium data were all fitted the Langmuir isotherm equation reasonably well, with a maximum adsorption capacity of 10.41 mg g(-1) for copper ions and of 217 m g g(-1) for RB5. A pseudo-second-order model also could best describe the adsorption kinetics, and the derived activation energy for copper ions and RB5 were 26.92 kJ mol(-1) and 12.06 kJ mol(-1), respectively. The optimum conditions to desorb cationic and anionic adsorbates from NH(2)/SiO(2)/Fe(3)O(4) were provided by a solution with 0.1M HNO(3) for copper ions and with 0.05 M NaOH for RB5.
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