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  • Title: Direct methoxypyridine functionalization approach to magellanine-type Lycopodium alkaloids.
    Author: Murphy RA, Sarpong R.
    Journal: Org Lett; 2012 Jan 20; 14(2):632-5. PubMed ID: 22201223.
    Abstract:
    A concise enantioselective approach to the tetracyclic core of the magellanine-type Lycopodium alkaloids is reported. Key to this approach is the use of the Hajos-Parrish reaction to set a challenging quaternary stereocenter, thereby guiding the stereoselectivity for the remainder of the synthesis, as well as the use of a palladium-mediated direct pyridine functionalization reaction to forge the tetracyclic core.
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