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  • Title: Self-assembled pit arrays as templates for the integration of Au nanocrystals in oxide surfaces.
    Author: Konstantinović Z, Sandiumenge F, Santiso J, Balcells L, Martínez B.
    Journal: Nanoscale; 2013 Feb 07; 5(3):1001-8. PubMed ID: 23250118.
    Abstract:
    We report on the fabrication of long-range ordered arrays of Au nanocrystals (sub-50 nm range) on top of manganite (La(2/3)Sr(1/3)MnO(3)) thin films achieving area densities around 2 × 10(10) gold nanocrystals per cm(2), well above the densities achievable by using conventional nanofabrication techniques. The gold-manganite interface exhibits excellent conduction properties. Long-range order is achieved by a guided self-assembling process of Au nanocrystals on self-organized pit-arrays acting as a template for the nucleation of gold nanocrystals. Self-organization of pits on the manganite film surface promoted by the underlying stepped SrTiO(3) substrate is achieved by a fine tuning of the growth kinetic pathway, taking advantage of the unusual misfit strain relaxation behaviour of manganite films.
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