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  • Title: Stereocontrolled total synthesis of hedyotol A.
    Author: Kawabe Y, Ishikawa R, Akao Y, Yoshida A, Inai M, Asakawa T, Hamashima Y, Kan T.
    Journal: Org Lett; 2014 Apr 04; 16(7):1976-9. PubMed ID: 24660822.
    Abstract:
    The total synthesis of hedyotol A (1), a natural product isolated from Hedyotis lawsoniae (DC.) Wight et Arn. (Rubiaceae), was accomplished in a highly stereocontrolled manner. Key steps include an L-proline-catalyzed cross-aldol reaction and the biomimetic construction of a furofuran lignan skeleton through a quinomethide intermediate.
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