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  • Title: Asymmetric synthesis of tetrahydroquinolines through a [3+2] cycloaddition controlled by dienamine catalysis.
    Author: Li W, Wei J, Jia Q, Du Z, Zhang K, Wang J.
    Journal: Chemistry; 2014 May 26; 20(22):6592-6. PubMed ID: 24789078.
    Abstract:
    A dienamine-mediated enantioselective 1,3-dipolar cycloaddition catalyzed by a chiral prolinol silyl ether catalyst has been developed. Removal of the benzamide group of the intermediates could furnish chiral C-1 substituted tetrahydroisoquinolines (see scheme) in high yields and excellent stereoselectivities.
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