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  • Title: MoS2-based nanoprobes for detection of silver ions in aqueous solutions and bacteria.
    Author: Yang Y, Liu T, Cheng L, Song G, Liu Z, Chen M.
    Journal: ACS Appl Mater Interfaces; 2015 Apr 15; 7(14):7526-33. PubMed ID: 25776005.
    Abstract:
    Silver as an extensively used antibacterial agent also poses potential threats to the environment and human health. Hence, in this work, we design a fluorescent nanoprobe by using rhodamine B isothiocyanate (RhoBS) adsorbed MoS2 nanosheets to realize sensitive and selective detection of Ag(+). On the surface of RhoBS-loaded MoS2 nanosheets, Ag(+) can be reduced to Ag nanoparticles, which afterward could not only lead to the detachment of RhoBS molecules and thus their recovered fluorescence but also the surface-enhanced fluorescence from RhoBS remaining adsorbed on MoS2. Such an interesting mechanism allows highly sensitive detection of Ag(+) (down to 10 nM) with great selectivity among other metal ions. Moreover, we further demonstrate that our MoS2-RhoBS complex could act as a nontoxic nanoprobe to detect Ag(+) in live bacteria samples. Our work resulted from an unexpected finding and suggests the promise of two-dimensional transition-metal sulfide nanosheets as a novel platform for chemical and biological sensing.
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