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  • Title: Total Synthesis of (+)-Rubriflordilactone A.
    Author: Goh SS, Chaubet G, Gockel B, Cordonnier MC, Baars H, Phillips AW, Anderson EA.
    Journal: Angew Chem Int Ed Engl; 2015 Oct 19; 54(43):12618-21. PubMed ID: 26337920.
    Abstract:
    Two enantioselective total syntheses of the nortriterpenoid natural product rubriflordilactone A are described, which use palladium- or cobalt-catalyzed cyclizations to form the CDE rings, and converge on a late-stage synthetic intermediate. These key processes are set up through the convergent coupling of a common diyne component with appropriate AB-ring aldehydes, a strategy that sets the stage for the synthetic exploration of other members of this family of natural products.
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