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  • Title: Efficient Strategy for the Construction of Both Enantiomers of the Octahydropyrroloquinolinone Ring System: Total Synthesis of (+)-Aspidospermidine.
    Author: Pandey G, Burugu SK, Singh P.
    Journal: Org Lett; 2016 Apr 01; 18(7):1558-61. PubMed ID: 26999058.
    Abstract:
    An efficient and highly stereoselective intramolecular [3 + 2] cycloaddition of nonstabilized azomethine ylide generated from a designed bicyclic aminal precursor is reported for the synthesis of both (-)- and (+)-octahydropyrroloquinolinone. One of the enantiomers is further advanced to accomplish the total synthesis of (+)-aspidospermidine.
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