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  • Title: Concentration-Gradient Multichannel Flow-Stream Membrane Capacitive Deionization Cell for High Desalination Capacity of Carbon Electrodes.
    Author: Kim C, Lee J, Srimuk P, Aslan M, Presser V.
    Journal: ChemSusChem; 2017 Dec 22; 10(24):4914-4920. PubMed ID: 28685992.
    Abstract:
    We present a novel multichannel membrane flow-stream capacitive deionization (MC-MCDI) concept with two flow streams to control the environment around the electrodes and a middle channel for water desalination. The introduction of side channels to our new cell design allows operation in a highly saline environment, while the feed water stream in the middle channel (conventional CDI channel) is separated from the electrodes with anion- and cation-exchange membranes. At a high salinity gradient between side (1000 mm) and middle (5 mm) channels, MC-MCDI exhibited an unprecedented salt-adsorption capacity (SAC) of 56 mg g-1 in the middle channel with charge efficiency close to unity and low energy consumption. This excellent performance corresponds to a fourfold increase in desalination performance compared to the state-of-the-art in a conventional CDI cell. The enhancement originates from the enhanced specific capacitance in high-molar saline media in agreement with the Gouy-Chapman-Stern theory and from a double-ion desorption/adsorption process of MC-MCDI through voltage operation from -1.2 to +1.2 V.
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