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  • Title: Two-tag correlations and nonequilibrium fluctuation-response relation in ageing single-file diffusion.
    Author: Ooshida T, Otsuki M.
    Journal: J Phys Condens Matter; 2018 Sep 19; 30(37):374001. PubMed ID: 30027890.
    Abstract:
    Spatiotemporally correlated motions of interacting Brownian particles, confined in a narrow channel of infinite length, are studied in terms of statistical quantities involving two particles. A theoretical framework that allows analytical calculation of two-tag correlations is presented on the basis of the Dean-Kawasaki equation describing density fluctuations in colloidal systems. In the equilibrium case, the time-dependent Einstein relation holds between the two-tag displacement correlation and the response function corresponding to it, which is a manifestation of the fluctuation-dissipation theorem for the correlation of density fluctuations. While the standard procedure of closure approximation for nonlinear density fluctuations is known to be obstructed by inconsistency with the fluctuation-dissipation theorem, this difficulty is naturally avoided by switching from the standard Fourier representation of the density field to the label-based Fourier representation of the vacancy field. In the case of ageing dynamics started from equidistant lattice configuration, the time-dependent Einstein relation is violated, as the two-tag correlation depends on the waiting time for equilibration while the response function is not sensitive to it. Within linear approximation, however, there is a simple relation between the density (or vacancy) fluctuations and the corresponding response function, which is valid even if the system is out of equilibrium. This non-equilibrium fluctuation-response relation can be extended to the case of nonlinear fluctuations by means of closure approximation for the vacancy field.
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