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  • Title: Distinctive distributions and migrations of 239+240Pu and 241Am in Chinese forest, grassland and desert soils.
    Author: Ni Y, Wang Z, Guo Q, Zheng J, Li S, Lin J, Tan Z, Huang W.
    Journal: Chemosphere; 2018 Dec; 212():1002-1009. PubMed ID: 30286529.
    Abstract:
    The vertical distributions and downward migrations of the global fallout derived 239+240Pu and 241Am in diverse types of Chinese soils (forest, grassland and desert) were studied. The mean 239+240Pu and 241Am activity concentrations in the investigated soil cores were 0.28-0.69 mBq/g and 0.13-0.37 mBq/g, respectively, while the accumulative inventories were 61.53-138.99 Bq/m2 for 239+240Pu and 28.29-61.05 Bq/m2 for 241Am. The convection-dispersion equation (CDE) was used to calculate the migration parameters of 239+240Pu and higher apparent dispersion coefficients (D) were observed for the acidic forest soils compared with the alkaline grassland and desert soils; meanwhile a compartment model was employed to compare the migration of 239+240Pu and 241Am in successive soil layers which showed that the migration behaviors of 239+240Pu and 241Am were rather similar; both velocities were less than 0.3 cm/y in diverse types of soils and these findings were compatible with those of short-term laboratory simulation experiments in China.
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