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  • Title: Adsorptive removal of strontium ions from aqueous solution by graphene oxide.
    Author: Xing M, Zhuang S, Wang J.
    Journal: Environ Sci Pollut Res Int; 2019 Oct; 26(29):29669-29678. PubMed ID: 31401804.
    Abstract:
    Graphene oxide (GO) was prepared, characterized, and applied for adsorption of Sr(II) in aqueous solution. The adsorption capacity was calculated to be 137.80 mg/g according to the Langmuir model. The observation by scanning electron microscope with energy dispersive X-ray detector (SEM-EDX), high-resolution transmission electron microscope (HRTEM), and X-ray diffraction (XRD) revealed the crystal structure of Sr compound on the surface of graphene sheets. The analyses by the Fourier transform infrared spectroscopy (FTIR) and X-ray photoelectron spectroscopy (XPS) indicated the involvement of O-C=O, C-O, and C-O-C groups during the adsorption. The X-ray absorption fine structure (XAFS) analysis provided the detail information of GO-Sr composites, and the fitting results were given by Sr(HCOO)2 and SrCO3 model, and the coordination numbers (CN) and interatomic distances (R) of Sr-O shell and Sr-C shell were calculated. The adsorption mechanism of Sr(II) was attributed to complexation between Sr and the acidic oxygen-containing groups, which lead to the agglomeration of graphene oxide. Two types of crystals were proposed. Type 1 was formed by coordination between Sr(II) and O-C=O groups, and type 2 was formed by coordination between Sr(II) and C-O/C-O-C groups.
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