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  • Title: CO2 hydrogenation by phosphorus-nitrogen PN3P-pincer iridium hydride complexes: elucidation of the deactivation pathway.
    Author: Pan Y, Guan C, Li H, Chakraborty P, Zhou C, Huang KW.
    Journal: Dalton Trans; 2019 Sep 14; 48(34):12812-12816. PubMed ID: 31402365.
    Abstract:
    PN3P-Ir pincer hydride complexes were synthesized and characterized as catalysts and key intermediates in the direct hydrogenation of CO2 to formate under mild conditions. The formation of a dearomatized PN3P*-Ir(i)-CO species was identified as a plausible key process accountable for the loss of catalytic activity in the CO2 hydrogenation.
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