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  • Title: Synergistic effects, gaseous products, and evolutions of NOx precursors during (co-)pyrolysis of textile dyeing sludge and bamboo residues.
    Author: Hu J, Song Y, Liu J, Evrendilek F, Buyukada M, Yan Y.
    Journal: J Hazard Mater; 2021 Jan 05; 401():123331. PubMed ID: 32652418.
    Abstract:
    This study aimed to investigate the synergistic influences of the textile dyeing sludge (TDS) and bamboo residues (BR) co-pyrolysis, and its effects on the formation mechanisms of NH3 and HCN. The mass loss rate was lower for TDS than BR, with the co-pyrolysis with 50% BR exerting the strongest synergistic effect. The pyrolysis stages 1 (< 400 °C) and 2 (400-800 °C) were best described using the diffusion and third-order reaction mechanisms, respectively. Activation energy and frequency factor were lower for the pyrolysis of TDS than BR. The addition of no less than 50% BR significantly increased the emissions of CO2, CO, CH4, CO, and CO and reduced the aromatic compounds. The thermal stability of N-A structure was lower in TDS than BR. The co-pyrolysis with 50% BR significantly inhibited the formations of NH3 and HCN and improved the aromaticity of biochar. This may due to the weakened hydrogenation reaction at N sites, the enhanced conversion of NH3, the inhibition of the ring cleavage in the char-secondary cracking, and the formation of more quaternary-N. Our results provide insights into the co-treatment of TDS and BR, and controls over NOx precursors for a cleaner energy production.
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