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  • Title: Distribution of tritium concentration in the 0-25 cm surface soil of cultivated and uncultivated soil around the Qinshan nuclear power plant in China.
    Author: Guo F, Wu W, Feng Y, Shen H.
    Journal: Appl Radiat Isot; 2020 Oct; 164():109311. PubMed ID: 32768888.
    Abstract:
    In this study, tritiated water (HTO) and organically bound tritium (OBT) activity concentration at different depth soil layers (0-5 cm, 5-10 cm, 10-15 cm, 15-20 cm, and 20-25 cm) were measured in uncultivated and cultivated soil samples collected in the vicinity of the Qinshan nuclear power plant (QNPP) in July, September, and December 2018. The concentration difference, the spatial and temporal distribution, the seasonal variation, and the OBT/HTO ratios were investigated. The average ratios of HTO concentration between uncultivated and cultivated soil moisture were 1.20 ± 0.24, 1.39 ± 0.46 and 0.95 ± 0.14 in July, September and December, respectively, the corresponding values for OBT were 1.17 ± 0.31, 1.22 ± 0.49 and 1.08 ± 0.28. In generally, the highest HTO concentration in uncultivated soil was found for the topsoil (0-5 cm) in July and September and for the deeper soil layer (20-25 cm) in December, while for cultivated soil, the highest levels were found for the middle layer soil in July, for the topsoil (0-5 cm) in September, and for the deeper layer soil (20-25 cm) in December. Both soils, the vertical profile distribution of OBT concentration showed no consistent tendency, and there were no significant differences in the HTO and OBT concentrations between different soil layers, except for the highest concentration. Whether uncultivated soil or cultivated soil, HTO activity concentrations showed an apparent spatial distribution and seasonal variability, decreasing with the distance to the release sources and with sampling time, while OBT concentrations showed lower spatial and seasonal variability than HTO. In most cases, the OBT/HTO ratios were less than 1, with average values of 1.01 ± 0.48 and 1.06 ± 0.86 for cultivated soil and cultivated soil samples, respectively. The results of this work suggest that farming may affect tritium behavior in soil, while the spatial and temporal distribution of tritium is only slightly impacted.
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