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  • Title: In situ fabrication of niobium pentoxide/graphitic carbon nitride type-II heterojunctions for enhanced photocatalytic hydrogen evolution reaction.
    Author: Dong Q, Chen Z, Zhao B, Zhang Y, Lu Z, Wang X, Li J, Chen W.
    Journal: J Colloid Interface Sci; 2022 Feb 15; 608(Pt 2):1951-1959. PubMed ID: 34749145.
    Abstract:
    The effective conversion of sunlight into H2 by photocatalytic water splitting has emerged as the most promising strategy to alleviate the energy crisis. In this work, niobium pentoxide (Nb2O5)/graphitic carbon nitride (g-C3N4) type-II heterojunctions with high photocatalytic H2 evolution rate under both visible and simulated solar light are fabricated via a novel approach involving in situ 'hydrolysis/calcination' loading of Nb2O5 nanoparticles on the g-C3N4 surface. After the optimisation, the Nb2O5/g-C3N4 heterojunctions with 5 wt% Nb2O5 content delivers high H2 evolution rates of 2.07 ± 0.03 and 6.77 ± 0.12 mmol g-1 h-1 under visible and simulated solar light exposure, respectively, which are 4.1 and 4.2 times superior to those of pure g-C3N4. According to the subsequent characterisations, the effective Nb2O5/g-C3N4 heterojunction offers sufficient contact interface, which is favourable for the efficient separation of photogenerated charges. In addition, the Nb2O5/g-C3N4 heterojunction possesses a large surface area, which contributes to the interfacial contact between photocatalyst and water. This work provides insights into the synthesis of novel g-C3N4-based hetero-photocatalysts with strong solar energy conversion capabilities.
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