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  • Title: Black Si-doped TiO2 nanotube photoanode for high-efficiency photoelectrochemical water splitting.
    Author: Dong Z, Ding D, Li T, Ning C.
    Journal: RSC Adv; 2018 Feb 02; 8(11):5652-5660. PubMed ID: 35539613.
    Abstract:
    Black Si-doped TiO2 (Ti-Si-O) nanotubes were fabricated through Zn metal reduction of the Ti-Si-O nanotubes on Ti-Si alloy in an argon atmosphere. The nanotubes were used as a photoanode for photoelectrochemical (PEC) water splitting. Both Si element and Ti3+/oxygen vacancies were introduced into the black Ti-Si-O nanotubes, which improved optical absorption and facilitated the separation of the photogenerated electron-hole pairs. The photoconversion efficiency could reach 1.22%, which was 7.18 times the efficiency of undoped TiO2. It demonstrated that a Si element and Ti3+/oxygen vacancy co-doping strategy could offer an effective method for fabricating a high-performance TiO2-based nanostructure photoanode for improving PEC water splitting.
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