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  • Title: Preparation and performance study of a PVDF-LATP ceramic composite polymer electrolyte membrane for solid-state batteries.
    Author: Liang X, Han D, Wang Y, Lan L, Mao J.
    Journal: RSC Adv; 2018 Dec 04; 8(71):40498-40504. PubMed ID: 35557886.
    Abstract:
    Recently, safety issues in conventional organic liquid electrolytes and the interface resistance between the electrode and electrolyte have been the most challenging barriers for the expansion of lithium batteries to a wide range of applications. Here, an ion-conductive PVDF-based composite polymer electrolyte (CPE) consisting of lithium aluminum germanium phosphate (Li1.3Al0.3Ti1.7(PO4)3) and polyvinylidene fluoride (PVDF) is prepared on a Li metal anode via a facile casting method. The ionic conductivity and electrochemical stability were enhanced by incorporating an appropriate amount of LATP into the PVDF-based composite polymer electrolyte, and the optimum content of LATP in the hybrid solid electrolyte was approximately 90 wt%. The corresponding solid-state battery based on an SEI-protected Li anode, the PVDF-LATP electrolyte, and a LiMn2O4 (LMO) cathode exhibited excellent rate capability and long-term cycling performance, with an initial discharge capacity of 107.4 mA h g-1 and a retention of 91.4% after 200 cycles.
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