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  • Title: Effects of organic carbon burial on biomarker component changes in contamination in northeast Dianchi watershed.
    Author: Chen Y, Zhao Z, Wang Y, Zhu W, Wu H, Zhang M, Zhang M.
    Journal: J Hazard Mater; 2023 Mar 05; 445():130474. PubMed ID: 36446312.
    Abstract:
    The upper reaches of the Yangtze River have experienced increasing anthropogenic stress. Quantitative tracing of carbon (C) sources and ecological risks through biomarkers i.e., polycyclic aromatic hydrocarbons (PAHs) and n-alkanes is significant for C neutrality and sequestration. Here, source and sink patterns, and factors influencing C burial and biomarker components in a small catchment of Dianchi Lake were explored. The sediment core covered the period 1855-2019. Before 1945, the organic C accumulation rate (OCAR) ranged from 0.71 to 5.12 mg cm-2 yr-1, and the PAHs and n-alkanes fluxes were 106.99-616.09 ng cm-2 yr-1 and 5.56-31.37 μg cm-2 yr-1. During 1945-2005, the OCAR, PAH, and n-alkane burial rapidly increased from 3.19 to 16.17 mg cm-2 yr-1, 230.40 to 2538.81 ng cm-2 yr-1, and 11.63 to 61.90 μg cm-2 yr-1. During 1855-2019, deposition fluxes of PAHs and n-alkanes increased 13.01 and 9.14 times, resulting in increased C burial, driven by environmental changes. A PMF model and the diagnostic ratio indicated that PAHs from coal combustion and traffic emission increased from 22.32% to 65.20% during 1855-2019. The PAH concentrations reflected normal-moderate contamination and potential risks to the aquatic environment. The results facilitate a comprehensive understanding of anthropogenic-driven interactions between increasing OC burial and ecological risks.
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