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  • Title: Spatial distribution, source identification, and transportation paths of plutonium in the Beibu Gulf, South China Sea.
    Author: Guan YJ, He H, Fan KD, Wang SZ, Guo ZC, Wang HJ, Cui LJ, Chen W, Huang CP, Liu ZY, He XW, Guo KX, Zhang JJ, Xu ZY.
    Journal: Mar Pollut Bull; 2024 Feb; 199():115972. PubMed ID: 38154170.
    Abstract:
    To investigate the spatial distribution and source of plutonium isotopes in the Beibu Gulf, surface sediments were collected and analyzed using sector field inductively coupled plasma mass spectrometry (SF-ICP-MS). The activities of 239+240Pu in surface sediments ranged from 0.012 to 0.451 mBq/g (mean: 0.171 ± 0.138 mBq/g, n = 36), indicating a decreasing trend in a counterclockwise direction from the southern bay mouth. The counterclockwise decreasing trend in the south of the bay mouth is similar to the current in the Beibu Gulf. The 240Pu/239Pu atom ratios in surface sediments ranged from 0.156 to 0.283 (mean: 0.236 ± 0.031, n = 36), slightly higher than that of the global fallout value of 0.18. This suggests that the Pu in the Beibu Gulf was a combination of global fallout and Pacific Proving Ground (PPG). The average contribution of the plutonium (Pu) derived from the PPG in the sediment was estimated to be 52 % ± 24 %.
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